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By RICHARD G. NELSON, MARIE WALSH, JOHN J. SHEEHAN,

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6 ps calculated for the core. In both cases, the slower decay is very close to the average decay of the primary charge separated state [P700+A0-] and the population of the first substantially irreversible charge separated state [P700+A1-]. This indicated that the kinetic of depopulation are strongly influenced by stable charge separations, but, at the same time, the antenna size influences the excited state lifetime. Thus, both of these factors contribute significantly to the excited state dynamics.

On the other hand, since in the simulations presented here the core and external antenna are considered separately, the transfer rate from the core to [RC*] is kept virtually to the same value (which is close to that estimated by Slavov and coworkers (2008)), while it is the coupling between the two antenna moieties which is varied. As mentioned above, up to physically reasonable rates for excited state transfer from (and to) the core antenna to (and from) the external antenna, we were required to increase of primary charge separation to preserve the population dynamics of [RC*].

E. the number of chromophore, in the antenna. Theoretical studies indicate that the trapping time of an iso-energetic lattice should scale linearly with the number of pigments. This can be understood in a simple intuitive manner considering that excitation losses increase proportionally to the number of steps in a random walk (Pealstain 1982, Kudsmauskas et al. 1983, Gobets et al. 2003b). However, this suggestion holds true principally when the energy transfer to the photochemical active centre represents the main kinetic limitation to the overall excited state dynamic, which is often referred to as a purely diffusion-limited model.

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